Relation between enthelpy of sublimation and rate of sublimation?

This conversation discusses the challenges of determining the sublimation rate of a material under high-temperature, high-vacuum conditions. The speaker mentions using the material's saturated vapor pressure to calculate the sublimation rate, but notes that this information is not available for the specific material they are working on. They also mention the enthalpy of sublimation, but have not found a direct relationship between it and the sublimation rate. Their question is whether such a relationship exists.
  • #1
DenisH
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TL;DR Summary
Is there a way to get the rate of sublimation of a material in vacuum for a given temperature from its enthalpy of sublimation?
Hello,
I am running experiments where materials are heated at high temperatures during tens of hours under high-vacuum conditions. Since what I am investigating lies in the first hundreds of nanometers of the materials, I must take into account (and anticipate) surface sublimation.
Therefore I am trying to determine at which rate a sample surface is sublimating. I found that this can be calculated from saturated vapor pressure, giving results in consistent with my experimental observations. Unfortunately for the material I am working on (UO2+x), no such saturated vapor pressure has ever been published... but enthalpy of sublimation had been.
At this stage I did not found a relation between enthalpy of sublimation and sublimation rate (or saturated vapor pressure)... my question thus is: is there one?
Thank you
 
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  • #2
DenisH said:
Summary:: Is there a way to get the rate of sublimation of a material in vacuum for a given temperature from its enthalpy of sublimation?

my question thus is: is there one?
No.
 
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